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Influence of Synthesis Conditions on the Capacitance Performance of Hydrothermally Prepared MnO2 for Carbon Xerogel-Based Solid-State Supercapacitors

Authors: Vania Ilcheva,Victor Boev,Mariela Dimitrova,Borislava Mladenova,Daniela Karashanova,Elefteria Lefterova,Natalia Rey-Raap,Ana Arenillas,Antonia Stoyanova
Publisher: MDPI AG
Publish date: 2025-1-15
ISSN: 2310-2861 DOI: 10.3390/gels11010068
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The reported electrochemical performance, particularly the 96% capacitance retention, seems unusually high and lacks independent verification or statistical validation. The crystallographic analysis is inconsistent, with insufficient details on Rietveld refinement parameters, and the claimed synergy between α-MnO2 and K1.39Mn3O6 is not convincingly demonstrated through proper control experiments. The study also lacks in-depth surface chemistry analysis (e.g., XPS or Raman spectroscopy) to confirm interactions between MnO2 and the carbon xerogel, leaving uncertainties about the actual mechanism. I encourage the authors to address these issues to strengthen the study’s rigor and improve the clarity and reliability of its findings.

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